Since you're looking for a front-end role, I'd say recommend showing off your best designed projects because regardless of implementation, similar to 'first impressions', your work needs to 'catch their eye.'
Aside from that, I'd research the technologies the company uses and leverage your experience with those technologies if they match up.
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Looking to transition from freelancing to being a full-time in-house front-end dev. What sort of work should I show on my portfolio?
Since you're looking for a front-end role, I'd say recommend showing off your best designed projects because regardless of implementation, similar to 'first impressions', your work needs to 'catch their eye.'
Aside from that, I'd research the technologies the company uses and leverage your experience with those technologies if they match up.